Session chairperson(s): Philipp del Hougne; Owen Miller
Session chairperson(s): Lucia Stein-Montalvo; Anastasiia O. Krushynska
Related publication: https://doi.org/10.1016/j.eml.2021.101510
https://arxiv.org/abs/2601.08866
See preprint https://arxiv.org/pdf/2601.00547
See our arXiv preprint: arxiv.org/abs/2511.22279
Controlling light-matter interactions at scales smaller than the diffraction limit at the single photon level is a critical challenge to advancing quantum technologies and sensing applications. Single-molecule nanophononics is an emerging field offering exciting opportunities to investigate light-matter interactions at the emitter level with nanometer-scale resolution.
We proposed a non-invasive methodology, capable of temporally and spatially correlating enhanced molecular single-emitter properties coupled to a novel material platform that enables precise engineering of spontaneous emission. This platform is based on freestanding hollow plasmonic nanocones arranged in a square lattice, uniformly scalable to the centimeter scale while maintaining unitary cell geometry. Exhibits diverse and tunable light-matter interaction enhancement properties in function of the out-of-plane illumination angle. Significantly increasing the local density of states (LDOS) in a manner that depends on both emitter position and dipole orientation, offering extreme position sensitivity within the 3D electromagnetic landscape. The strong changes in the emission of molecular single emitters along the 3D nanofields in the metamaterial, leads to billions of Purcell-enhanced single emitters integrated into a single nanodevice. We measured the LDOS modification along the 3D fields with nano precision and single emitter level. Implementing a non-scanning widefield method combining far-field single-molecule super-resolution microscopy, with time correlation single photon counting (TCSPC), we probe molecule per molecule enhanced quantum light-matter interactions.
These unique properties offer an exceptionally sensitive platform for molecular sensing and the detection of small vectorial field variations with resolution surpassing the diffraction limit. By leveraging these plasmonic nanostructures and our method for measuring single-molecule Purcell-enhanced nano-resolved maps, we enable fine-tuned control of light-matter interactions. Obtaining fast single-photon sources at room temperature, provides a powerful tool for quantum applications at the single-emitter level. Our results heralds advances in technologies limited by resolution, single-photon efficiency, sensitive detection, scalability, low-density sensing, and vectorial field mapping.
Metasurfaces have been attracting tremendous attention from both the scientific community and industry in recent years. Due to their ability to efficiently control phase, amplitude and polarization of light at the nanoscale, they can be designed to perform a variety of optical functions and substitute conventional bulk optics with thinner flat optical components with enhanced functionality. However, to make their way to real products, the development of foundry-type large-scale manufacturing of metasurfaces with fixed PDKs is of primarily importance. In this talk, I will share our recent progress in development of large-scale manufacturing of dielectric metasurfaces using 12-inch wafer processing and their applications to passive and active flat optics-based devices, including wide field of view metalenses, RGB imaging cameras, 1-micron pixel liquid crystal on silicon meta-displays and more.
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